Didn’t tryed this, and I’m just guessing what you want to acomplish, but here it is:
int[] arrayRow;
int[] arrayCol;
int[,] myArray = new int[Math.Max(arrayRow.Length, arrayCol.Length), 2];
for (int i = 0; i < arrayRow.Length; i++)
myArray[i, 0] = arrayRow[i];
for (int i = 0; i < arrayCol.Length; i++)
myArray[i, 1] = arrayCol[i];
solved Combining two single dimensional arrays in a 2D array in c#